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Spatiotemporal patterns, loads, and risks of microplastics in the stormwater system of a subtropical coastal city

datacite.subject.sdg06:Água Potável e Saneamento
datacite.subject.sdg11:Cidades e Comunidades Sustentáveis
datacite.subject.sdg12:Produção e Consumo Sustentáveis
dc.contributor.authorDu, Aolei
dc.contributor.authorXu, Youxiang
dc.contributor.authorLuo, Yutang
dc.contributor.authorJian, Qiying
dc.contributor.authorLi, Yanjun
dc.contributor.authorZhan, Ziying
dc.contributor.authorQiu, Sizhe
dc.contributor.authorKam, Chon Wa
dc.contributor.authorChan, Tin-Chak
dc.contributor.authorHuang, Tsz-Yin
dc.contributor.authorPower, Deborah Mary
dc.contributor.authorZhang, Kai
dc.date.accessioned2026-08-24T12:49:27Z
dc.date.available2026-08-24T12:49:27Z
dc.date.issued2026-09
dc.description.abstractUrban stormwater runoff is a critical pathway for microplastics (MPs) to enter marine ecosystems, posing a significant threat. However, systematic studies on spatiotemporal patterns, loads, and risks of MPs in stormwater systems, particularly in subtropical coastal cities, remain limited. This study characterized MPs in Macao's stormwater drains across seasons, using density separation, H2O2 digestion, stereomicroscopy, and μ-FTIR analysis to investigate their abundance and distribution. MPs were ubiquitous across all sample sites, with abundance ranging from 0.86 to 53.03 n/L. Irregular shaped fragments (56.78 ± 0.13.80%) and the color black (38.44 ± 7.47%) were dominant, and the most common polymers were Polyethylene terephthalate (39.55 ± 16.63%), polypropylene (23.05 ± 18.15%), and polyethylene (9.52 ± 8.87%). While abundance of MPs was higher in the wet season, no significant seasonal variation was found. MP characteristics varied significantly with land use. The concentration range of MPs was estimated to be from 2.86 ± 0.38 to 3145.94 ± 766.74 μg/L, with an overall mean of 454.68 ± 572.20 μg/L through the mass concentration models. The daily MP emission load into the receiving water was estimated to range from 8.29 × 103 to 3.09 × 108 particles per day or 2.66 to 10,365.23 g/day. MP risk was high (Polymer Hazard Index/Potential Ecological Risk Index: III/V) due to hazardous polymers, with spatiotemporal variations further observed from fluctuating water flow erosion. Correlation analysis revealed that MP abundance showed a significant negative correlation with dissolved oxygen and a positive correlation with antecedent rainfall. These findings identify stormwater drains as a key MP conduit, influenced by rainfall and land use, calling for targeted management in urban coastal areas.eng
dc.identifier.doi10.1016/j.emcon.2026.100706
dc.identifier.issn2405-6650
dc.identifier.urihttp://hdl.handle.net/10400.1/29316
dc.language.isoeng
dc.peerreviewedyes
dc.publisherElsevier BV
dc.relation.ispartofEmerging Contaminants
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
dc.titleSpatiotemporal patterns, loads, and risks of microplastics in the stormwater system of a subtropical coastal cityeng
dc.typejournal article
dspace.entity.typePublication
oaire.citation.issue3
oaire.citation.startPage100706
oaire.citation.titleEmerging Contaminants
oaire.citation.volume12
oaire.versionhttp://purl.org/coar/version/c_970fb48d4fbd8a85
person.familyNamePower
person.givenNameDeborah Mary
person.identifier.ciencia-id891A-8A44-3CAE
person.identifier.orcid0000-0003-1366-0246
person.identifier.scopus-author-id7101806760
relation.isAuthorOfPublicationc68f5ffb-63f6-4c70-8957-29e464fb59c0
relation.isAuthorOfPublication.latestForDiscoveryc68f5ffb-63f6-4c70-8957-29e464fb59c0

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